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Percolative transition on ferromagnetic insulator manganites: Uncorrelated to correlated polaron clusters

Title
Percolative transition on ferromagnetic insulator manganites: Uncorrelated to correlated polaron clusters
Type
Article in International Scientific Journal
Year
2006
Authors
Lopes, Anabela M L M L M L
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Araújo, João Pedro
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Ramasco, José J.
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Suryanarayanan, Ramanathaan
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Correia, J. G.
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Authenticus ID: P-004-N4D
Abstract (EN): We report an atomic-scale study on the ferromagnetic insulator manganite LaMnO3.12 using gamma-gamma perturbed angular correlation spectroscopy. Data analysis reveals a nanoscopic transition from an undistorted to a Jahn-Teller (JT) distorted local environment upon cooling. The percolation thresholds of the two local environments enclose a macroscopic structural transition (rhombohedral-orthorhombic). Two distinct regimes of JT distortions were found: a high-temperature regime where uncorrelated polaron clusters with severe distortions of the Mn3+O6 octahedra survive up to T approximate to 800 K and a low-temperature regime where correlated regions have a weaker JT-distorted symmetry.
Language: English
Type (Professor's evaluation): Scientific
Contact: armandina.lima.lopes@cern.ch
No. of pages: 4
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