Abstract (EN):
We report an atomic-scale study on the ferromagnetic insulator manganite LaMnO3.12 using gamma-gamma perturbed angular correlation spectroscopy. Data analysis reveals a nanoscopic transition from an undistorted to a Jahn-Teller (JT) distorted local environment upon cooling. The percolation thresholds of the two local environments enclose a macroscopic structural transition (rhombohedral-orthorhombic). Two distinct regimes of JT distortions were found: a high-temperature regime where uncorrelated polaron clusters with severe distortions of the Mn3+O6 octahedra survive up to T approximate to 800 K and a low-temperature regime where correlated regions have a weaker JT-distorted symmetry.
Language:
English
Type (Professor's evaluation):
Scientific
Contact:
armandina.lima.lopes@cern.ch
No. of pages:
4