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Substitutional disorder and charge localization in manganites

Title
Substitutional disorder and charge localization in manganites
Type
Article in International Scientific Journal
Year
2010
Authors
Lopes dos Santos, JMBL
(Author)
FCUP
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Journal
Vol. 22
Final page: 075601
ISSN: 0953-8984
Scientific classification
FOS: Natural sciences > Physical sciences
Other information
Authenticus ID: P-003-933
Abstract (EN): In the manganites RE(1-x)AE(x)MnO(3) (RE and AE being rare-earth and alkaline-earth elements, respectively) the random distribution of RE3+ and AE(2+) induces random, but correlated, shifts of site energies of charge carriers in the Mn sites. We consider a realistic model of this diagonal disorder, in addition to the double-exchange hopping disorder, and investigate the metal-insulator transition as a function of temperature, across the paramagnetic-ferromagnetic line, and as a function of doping x. Contrary to previous results, we find that values of parameters, estimated from the electronic structure of the manganites, are not incompatible with the possibility of a disorder-induced metal to insulator transition accompanying the ferromagnetic to paramagnetic transition at intermediate doping (x similar to 0.2-0.4). These findings indicate clearly that substitutional disorder has to be considered as an important effect when addressing the colossal magnetoresistance properties of manganites.
Language: English
Type (Professor's evaluation): Scientific
Contact: evcastro@fc.up.pt
No. of pages: 5
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