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Control of efficiency of photon energy up-conversion in CdSe/ZnS quantum dots

Title
Control of efficiency of photon energy up-conversion in CdSe/ZnS quantum dots
Type
Article in International Scientific Journal
Year
2003
Authors
Rusakov, KI
(Author)
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Gladyshchuk, AA
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Rakovich, YP
(Author)
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Donegan, JF
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Filonovich, SA
(Author)
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Gomes, MJM
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Talapin, DV
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Rogach, AL
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Eychmuller, A
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Journal
The Journal is awaiting validation by the Administrative Services.
Vol. 94
Pages: 859-863
ISSN: 0030-400X
Other information
Authenticus ID: P-000-GHE
Abstract (EN): Efficient photoluminescence (PL) up-conversion in CdSe/ZnS quantum dots prepared by an organometallic approach is reported. It is demonstrated that the efficiency of photon energy up-conversion and the magnitude of the spectral shift can be controlled by (i) the thickness of the ZnS layers, (ii) the temperature dependence of the excited-state absorption coefficient, and (iii) the dependence on the excitation intensity. From the analysis of the experimental data, it is proposed that intrinsic gap states are involved as intermediate states in the PL up-conversion, rather than nonlinear two-photon absorption or Auger processes. (C) 2003 MAIK "Nauka/Interperiodica".
Language: English
Type (Professor's evaluation): Scientific
No. of pages: 5
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Control of efficiency of photon energy up-conversion in CdSe/ZnS quantum dots (2003)
Article in International Scientific Journal
Rusakov, KI; Gladyshchuk, AA; Rakovich, YP; Donegan, JF; Filonovich, SA; Gomes, MJM; Talapin, DV; Rogach, AL; Eychmuller, A
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