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Thermodynamics of long-chain 1-alkyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide ionic liquids

Title
Thermodynamics of long-chain 1-alkyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide ionic liquids
Type
Article in International Scientific Journal
Year
2016
Authors
Paulechka, E
(Author)
Other
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Blokhin, AV
(Author)
Other
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Rodrigues, ASMC
(Author)
Other
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Rocha, MAA
(Author)
Other
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Journal
Vol. 97
Pages: 331-340
ISSN: 0021-9614
Publisher: Elsevier
Other information
Authenticus ID: P-00K-87X
Abstract (EN): The heat capacities in the temperature range (5 to 370) K and the parameters of solid-phase transitions and fusion were determined for three [C(n)mim][NTf2] (n = 10, 14, 16) ILs. The temperature-dependent vapour pressures of [C(14)mim][NTf2] and [C(16)mim][NTf2] were measured with a Knudsen effusion apparatus combined with a quartz crystal microbalance. Thermodynamic properties of these compounds in the crystal, liquid, and gas states were derived from the obtained data. The results obtained in this work were combined to those available in the literature for the short-chain homologues to discuss regularities in thermodynamic properties of the series. While some properties demonstrate simple linear dependence on the alkyl chain length, a more complicated behaviour with strong non-linearity or a break at n = 6 is observed for others. Published by Elsevier Ltd.
Language: English
Type (Professor's evaluation): Scientific
No. of pages: 10
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