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A Complete Separation of Hexane Isomers by a Functionalized Flexible Metal Organic Framework

Title
A Complete Separation of Hexane Isomers by a Functionalized Flexible Metal Organic Framework
Type
Article in International Scientific Journal
Year
2014
Authors
Patrícia A. P. Mendes
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Patricia Horcajada
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Sébastien Rives
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Hong Ren
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Alírio E. Rodrigues
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Thomas Devic
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Emmanuel Magnier
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Philippe Trens
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Hervé Jobic
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Jacques Ollivier
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Guillaume Maurin
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Christian Serre
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José A. C. Silva
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Journal
Vol. 24 No. 48
Pages: 7666-7673
ISSN: 1616-301X
Publisher: Wiley-Blackwell
Other information
Authenticus ID: P-00A-2RD
Abstract (EN): The separation ability of branched alkane isomers (nHEX, 3MP, 22DMB) of the flexible and functionalized microporous iron(III) dicarboxylate MIL-53(Fe)-(CF3)(2) solid is evaluated through a combination of breakthrough experiments (binary or ternary mixtures), adsorption isotherms, X-ray diffraction temperature analysis, quasi-elastic neutron scattering measurements and molecular dynamics simulations. A kinetically controlled molecular sieve separation between the di-branched isomer of hexane 22DMB from a mixture of paraffins is achieved. The reported total separation between mono-and di-branched alkanes which was neither predicted nor observed so far in any class of porous solids is spectacular and paves the way towards a potential unprecedented upgrading of the RON of gasoline.
Language: English
Type (Professor's evaluation): Scientific
No. of pages: 8
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